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Rheology and Thixotropy

My research in rheology and thixotropy focuses on the mathematical and computational modelling of complex materials whose flow resistance and internal structure evolve with deformation and time. This work combines non-Newtonian fluid mechanics, constitutive modelling and numerical simulation to investigate the transport and deposition of sediment-rich and tailings materials.

A central aspect of my work is thixotropy: the time-dependent breakdown of material structure under shearing and its gradual recovery during periods of rest. These processes can strongly influence viscosity, yield stress, flow depth, velocity, runout distance, channel formation and the final geometry of deposited material.

I develop numerical models in which the Navier–Stokes equations are coupled with constitutive rheological relations and a transported structural parameter. This enables the material properties to evolve dynamically according to the local shear conditions and deformation history rather than being prescribed as constant values.

My work includes the implementation and comparison of different thixotropic formulations, including the Houska and Parent–Simms models, within free-surface flow simulations. Particular attention is given to numerical stability, fully implicit time integration, generalized coordinate systems, finite-volume discretization, adaptive free-surface grids and efficient multigrid solution methods.

The broader objective is to improve the physical realism and predictive capability of computational models for treated tailings, sediment–water mixtures and other complex fluids in which rheology evolves during transport, deposition and periods of rest.

Advanced Rheology and Thixotropy

My research addresses an important limitation of conventional flow-modelling approaches: time-dependent thixotropic behaviour is generally not represented in the standard rheological formulations used in conventional hydraulic and CFD modelling. This is particularly important for treated tailings and sediment-rich mixtures, where material structure can break down under shear and rebuild during periods of rest, substantially changing the subsequent flow and deposition behaviour.

I develop numerical models that couple the governing flow equations with constitutive rheological models and a dynamically evolving structural parameter. This allows viscosity, yield behaviour and material strength to evolve according to both the instantaneous flow conditions and the deformation history of the material.

The resulting framework provides capabilities beyond conventional time-independent rheological modelling. It enables direct investigation of how structural breakdown, recovery, shear history and changing rheology influence free-surface flow, runout and deposition. The integration of these processes within a fully coupled numerical flow model makes this research a distinctive and innovative contribution to computational rheology and thixotropic-flow modelling.

Areas of Expertise

Rheology and Thixotropic Behaviour

My expertise covers the physical and mathematical modelling of non-Newtonian and thixotropic materials, with particular emphasis on materials whose flow resistance, viscosity and internal structure evolve with deformation and time.

  • Non-Newtonian fluid mechanics
  • Time-dependent rheological behaviour
  • Thixotropy and structural evolution
  • Shear-rate-dependent viscosity
  • Constitutive rheological modelling
  • Houska thixotropic model
  • Parent–Simms thixotropic model
  • Coupling of rheology with flow dynamics
  • Free-surface flow of complex fluids
  • Flow and deposition of treated tailings
  • Sediment-rich and water–soil mixtures

A particular focus of my work is the coupling between material structure and flow. The local deformation history determines the evolution of the material structure and rheological properties, while those changing properties subsequently modify the velocity, stresses and overall flow behaviour. This two-way interaction is essential for realistically modelling thixotropic materials during transport, deposition, rest and remobilisation.

Computational Modelling of Thixotropic Flows

I develop numerical models for thixotropic free-surface flows in which fluid dynamics and time-dependent material behaviour are solved as a coupled system. The flow equations are combined with structural evolution equations so that the rheological properties evolve continuously according to the local deformation and shear history of the material.

  • Coupled flow and thixotropy equations
  • Transport equations for structural parameters
  • Time-dependent viscosity and yield behaviour
  • 2DV Navier–Stokes-based flow formulation
  • Applied Finite Volume Method (FVM)
  • Generalized and curvilinear coordinate systems
  • Implicit time integration
  • Adaptive treatment of the free surface
  • Geometric multigrid solution methods
  • Numerical treatment of strongly varying viscosity
  • Normalization

A distinctive aspect of this work is the direct coupling between flow dynamics and the evolving material structure. The model can therefore represent how shearing changes the material properties during motion, how structure recovers during periods of rest, and how these changes subsequently influence flow, free-surface evolution and deposition.

Material structure → Rheological behaviour → Constitutive model → Structural evolution → Flow dynamics → Free-surface transport → Deposition and recovery

From Rheological Behaviour to Thixotropic Flow Simulation

Thixotropic flow modelling connects the physical behaviour of complex materials with constitutive rheology, structural evolution and computational fluid dynamics. My work covers this complete modelling chain, from understanding how material structure responds to deformation to simulating the resulting free-surface flow, spreading and deposition.

  1. The rheological behaviour of the material is characterized, including yield behaviour, shear-dependent viscosity, structural breakdown under deformation and structural recovery during periods of rest.
  2. The material behaviour is formulated mathematically using appropriate constitutive rheological relations together with a structural parameter that represents the evolving state of the material.
  3. A structural evolution equation is coupled with the governing flow equations, allowing the rheological properties to evolve dynamically according to the local shear conditions and deformation history.
  4. The coupled flow and thixotropy equations are discretized and solved numerically, including the treatment of strongly varying viscosity, free-surface deformation and nonlinear material behaviour.
  5. The resulting model is used to investigate how thixotropy influences flow mobility, velocity, free-surface evolution, spreading, deposition, stopping and subsequent remobilisation.

My expertise therefore combines physical rheology, non-Newtonian fluid mechanics, constitutive modelling, numerical methods and free-surface flow simulation. The key distinction is that the material properties are not treated as fixed or determined only by the instantaneous flow conditions. Instead, the model accounts for the evolving structural state and the deformation history of the material.

Non-Newtonian flow Thixotropy Yield stress Time-dependent rheology Houska model Parent–Simms model Constitutive modelling Free-surface flow Finite volume Implicit time integration Multigrid Tailings deposition

Research Projects and Applications

01 · Rijpdijk Pilot

Simulation of Thixotropic Clay Flow over a Dike

In the Rijpdijk project, I applied a two-dimensional vertical (2DV) curvilinear free-surface flow model to simulate the gravity-driven movement of clay-rich material from the crest of a dike towards the collection pond at its toe.

The numerical model combines free-surface hydrodynamics with time-dependent rheology. The material structure evolves according to the local deformation and shear history, allowing changes in viscosity and flow resistance to develop dynamically as the clay moves down the slope.

The curvilinear formulation enables the computational grid to follow the dike geometry and the evolving free surface. This provides a physically based framework for investigating flow velocity, flow depth, spreading and deposition over the complete dike profile.

  • Two-dimensional vertical (2DV) modelling
  • Boundary-fitted curvilinear coordinates
  • Free-surface flow
  • Gravity-driven clay flow
  • Non-Newtonian rheology
  • Thixotropic material behaviour
  • Time-dependent viscosity and flow resistance
  • Structural breakdown under shear
  • Structural recovery
  • Shear-history effects
  • Finite Volume Method
  • Moving free-surface grid
  • Flow-depth and velocity evolution
  • Downslope spreading
  • Deposition towards the collection pond
  • Comparison with field-scale observations

From Dike Crest to Collection Pond

Clay-rich material is introduced near the crest of the dike and accelerates downslope under gravity. During this motion, the material undergoes continuous deformation, causing its structural state and rheological properties to evolve.

Farther downslope, changes in geometry, flow depth and material rheology influence the mobility of the clay. The flow gradually spreads and decelerates as it approaches the lower part of the dike and the collection pond.

Field-Scale Rheological Application

The project provides an opportunity to connect rheological characterization with field-scale flow behaviour. Material parameters obtained from measurements can be introduced into the numerical formulation, while calculated velocities, flow depths, spreading and deposited profiles can be compared with observations from the Rijpdijk experiment.

This creates a direct link between material rheology and engineering- scale behaviour, enabling the influence of thixotropy on the mobility, spreading and final deposition of clay to be investigated under realistic dike-scale conditions.

Clay placement → Gravity-driven flow → Shearing and structural evolution → Changing rheology → Downslope spreading → Deceleration → Deposition → Collection pond
images/rijpdijk.png

Field-scale clay flow from the crest of the dike towards the collection pond.

Numerical Simulation

Numerical simulation of gravity-driven thixotropic clay flow from the crest of the dike towards the collection pond.

02 · Tailings Deposition and Management

Thixotropic Modelling of Treated-Tailings Deposition Flows

This research investigates the influence of time-dependent rheology on the flow and deposition of treated tailings. Flocculated fine tailings can exhibit pronounced thixotropic behaviour: their internal structure changes during shearing and can recover during periods of rest, causing the apparent viscosity and flow resistance to evolve continuously during deposition.

I developed and applied a free-surface numerical flow model in which the governing fluid-flow equations are coupled with time-dependent rheological formulations. This enables the material structure and rheological properties to evolve dynamically as the tailings are transported and deposited.

Why Time-Dependent Rheology Matters

Conventional time-independent rheological models assume that the material response is determined by the instantaneous flow conditions. For thixotropic tailings, however, the current material properties also depend on the preceding shear and rest history.

The simulations demonstrate that the choice of thixotropic formulation can influence predicted flow depth, flow velocity and free-surface behaviour. Representing this time dependency is therefore important when predicting the spreading and deposition of treated tailings.

  • Flocculated and treated tailings
  • Non-Newtonian free-surface flow
  • Time-dependent rheology
  • Thixotropic material behaviour
  • Structural breakdown under shear
  • Structural recovery during rest
  • Shear-history effects
  • Transported structural parameters
  • Houska thixotropic formulation
  • Parent–Simms thixotropic formulation
  • Comparison of constitutive models
  • Spatially and temporally varying viscosity
  • Free-surface flow simulation
  • Flow-depth prediction
  • Velocity prediction
  • Deposition-flow behaviour
  • Flocculation effects
  • Runout and spreading behaviour

Comparison of Thixotropic Models

An important part of the work was the comparison of different constitutive descriptions of thixotropy. The Houska and Parent–Simms approaches were implemented within the numerical flow framework and evaluated for flocculated mature fine tailings.

The comparison showed that different representations of structural evolution can produce different predictions of flow depth, velocity and free-surface behaviour. The work therefore provides insight not only into tailings deposition itself, but also into the consequences of selecting a particular constitutive description for time-dependent material behaviour.

Deposition Behaviour and Free-Surface Dynamics

The later phase of the research examined time-dependent behaviour in tailings deposition flows more broadly. The calculations investigated how changes in rheological properties and flow conditions influence the evolution of the free surface and the behaviour of material during deposition.

The work also examined the role of flocculation. Because flocculation changes the rheological properties of fine tailings, it can influence predicted stream depth and flow velocity and may consequently affect the development and runout of deposition flows.

Flocculation → Material structure → Shear-induced breakdown and recovery → Time-dependent rheology → Free-surface flow → Spreading and deposition

Application to Tailings Management

The practical objective is to improve the physical basis of numerical tools used to understand and predict tailings deposition. Better representation of time-dependent rheology can support assessment of how treated tailings spread, develop flow paths and establish their deposited geometry.

The project therefore connects fundamental rheological behaviour with an important engineering application: improving physics-based prediction of deposition processes in tailings storage facilities.

Simulation

Numerical modelling of free-surface tailings flow with time-dependent rheological behaviour.

Publications

The subsequent research was published as: “Comparing various thixotropic models and their performance in predicting flow behaviour of treated tailings”, published in the proceedings of Paste 2023, Banff, Canada.

“Exploring the role of time-dependency in tailings deposition flows”, published in the proceedings of the 26th International Conference on Paste, Thickened and Filtered Tailings (Paste 2024), pages 257–270.

From Fundamental Rheology to Predictive Flow Modelling

My work bridges fundamental rheological behaviour and practical numerical modelling of complex, time-dependent materials. At the fundamental level, the focus is on understanding how shear, deformation history and periods of rest influence material structure, viscosity, yield behaviour and flow resistance.

These physical processes are incorporated into computational models through constitutive relations and structural-evolution equations coupled directly to the governing flow equations. This allows the material properties to evolve dynamically during transport, deposition, rest and remobilisation, rather than being represented by fixed or purely instantaneous rheological parameters.

The broader value of this modelling approach lies in:

Material structure → Shear and deformation history → Structural breakdown and recovery → Evolving rheology → Coupled flow simulation → Spreading and deposition → Predictive thixotropic modelling

Overall Rheology and Thixotropy Expertise

My expertise spans the complete modelling chain for non-Newtonian and thixotropic flows, from understanding the underlying material physics and constitutive behaviour to developing coupled numerical models for time-dependent flow, free-surface evolution and deposition.

Material structure → Rheological behaviour → Structural breakdown and recovery → Constitutive modelling → Coupled flow equations → Free-surface dynamics → Deposition and remobilisation
Rheology Non-Newtonian flows Thixotropy Time-dependent rheology Yield-stress fluids Shear-rate dependence Viscosity evolution Shear-history effects Structural breakdown Structural recovery Structural parameter Structural evolution equations Constitutive modelling Houska model Parent–Simms model Free-surface flow Treated tailings Sediment-rich mixtures

This combination enables me to investigate complex fluids from the evolution of their internal material structure to their large-scale flow, spreading, stopping and deposition behaviour.

A central theme of my work is that the rheological properties of a thixotropic material cannot always be regarded as fixed. The material continuously evolves as it is sheared, transported, deposited and allowed to rest. Its present flow behaviour can therefore depend strongly on its previous deformation history.

My work integrates rheological physics, constitutive modelling, computational fluid dynamics and numerical-method development to represent this history-dependent behaviour directly within flow simulations. This provides a more physically based framework for investigating treated tailings and other complex materials whose properties evolve during motion and rest.